Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
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Title:
Enhancement of hydrogen gas permeability in electrically aligned MWCNT-PMMA composite membranes
Authors:
Kumar, S; Sharma, A; Tripathi, B; Srivastava, S; Agrawal, S; Singh, M; Awasthi, K; Vijay, YK
Author Full Names:
Kumar, Sumit; Sharma, Anshu; Tripathi, Balram; Srivastava, Subodh; Agrawal, Shweta; Singh, M.; Awasthi, Kamlendra; Vijay, Y. K.
Source:
MICRON 41 (7): 909-914 OCT 2010
Language:
English
Document Type:
Review
Author Keywords:
MWCNT; PM MA; Membrane; Electrical field alignment; Gas permeation; Raman spectroscopy; XRD
KeyWords Plus:
WALL CARBON NANOTUBES; FAST MASS-TRANSPORT; SEPARATION MEMBRANES; POLYMER COMPOSITES; FIELD; PERMEATION; STORAGE; ADSORPTION
Abstract:
The multi-walled carbon nanotube (MWCNT) dispersed polymethylmethacrylate (PMMA) composite membranes have been prepared for hydrogen gas permeation application. Composite membranes are characterized by Raman spectroscopy, optical microscopy, X-ray diffraction, electrical measurements and gas permeability measurements. The effect of electric field alignment of MWCNT in PMMA matrix on gas permeation has been studied for hydrogen gas. The permeability measurements indicated that the electrically aligned MWCNT in PMMA has shown almost 2 times higher permeability for hydrogen gas as compare to randomly dispersed MWCNT in PMMA. The enhancement in permeability is explained on the basis of well aligned easy channel provided by MWCNT in electrically aligned sample. The effect of thickness of membrane on the gas permeability also studied and thickness of about 30 mu m found to be optimum thickness for fast hydrogen gas permeates. (C) 2010 Elsevier Ltd. All rights reserved.
Reprint Address:
Kumar, S, Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India.
Research Institution addresses:
[Kumar, Sumit; Sharma, Anshu; Tripathi, Balram; Srivastava, Subodh; Agrawal, Shweta; Singh, M.; Vijay, Y. K.] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India; [Awasthi, Kamlendra] Indian Inst Technol, Dept Chem Engn, DST Unit Nanosci, Kanpur 208016, Uttar Pradesh, India
E-mail Address:
sumitphy11@gmail.com; yk_vijay@sancharnet.in
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Cited Reference Count:
38
Times Cited:
0
Publisher:
PERGAMON-ELSEVIER SCIENCE LTD; THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
Subject Category:
Microscopy
ISSN:
0968-4328
DOI:
10.1016/j.micron.2010.05.016
IDS Number:
652GX
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Title:
Water Diffusion Behaviors and Transportation Properties in Transmembrane Cyclic Hexa-, Octa- and Decapeptide Nanotubes
Authors:
Liu, JA; Fan, JF; Tang, M; Cen, M; Yan, JF; Liu, Z; Zhou, WG
Author Full Names:
Liu, Jian; Fan, Jianfen; Tang, Min; Cen, Min; Yan, Jianfeng; Liu, Zhao; Zhou, Weigun
Source:
JOURNAL OF PHYSICAL CHEMISTRY B 114 (38): 12183-12192 SEP 30 2010
Language:
English
Document Type:
Article
KeyWords Plus:
ASSEMBLING PEPTIDE NANOTUBES; MOLECULAR-DYNAMICS; CARBON NANOTUBES; LIPID-BILAYER; LIQUID WATER; CHANNELS; PERMEATION; ION; MEMBRANES; MODEL
Abstract:
Molecular dynamics simulations have been performed on three transmembrane cyclic peptide nanotubes, i.e., 8 x (W (L) under barL)(n=345)/POPE (with uniform lengths but various radii) to investigate the radial dependences of the water-chain structures, diffusions, and transportation properties. The diffusions of individual water molecules and collective coordinates of all the channel-water in the three systems are certified as unbiased Brownian motions. From the very good linear relationships between MSDs and time intervals, the diffusion coefficients and transportation permeabilities have been deduced efficiently. Under the hydrostatic pressure differences across the membrane, a net unidirectional water flow rose up, and the osmotic permeabilities were determined. The ratios of the osmotic and diffusion permeabilities (p(f)/p(d)) were examined for all the three channels.
Reprint Address:
Fan, JF, Soochow Univ, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China.
Research Institution addresses:
[Liu, Jian; Fan, Jianfen; Tang, Min; Cen, Min; Zhou, Weigun] Soochow Univ, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China; [Yan, Jianfeng; Liu, Zhao] Soochow Univ, Sch Comp Sci & Technol, Suzhou 215006, Peoples R China
E-mail Address:
jffan1305@163.com
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Cited Reference Count:
54
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Physical
ISSN:
1520-6106
DOI:
10.1021/jp1039207
IDS Number:
652OV
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Title:
Desalination-of water by vapor-phase transport through hydrophobic nanopores
Authors:
Lee, J; Karnik, R
Author Full Names:
Lee, Jongho; Karnik, Rohit
Source:
JOURNAL OF APPLIED PHYSICS 108 (4): Art. No. 044315 AUG 15 2010
Language:
English
Document Type:
Article
KeyWords Plus:
REVERSE-OSMOSIS MEMBRANES; CONDENSATION COEFFICIENT; EVAPORATION COEFFICIENT; CARBON NANOTUBE; SEAWATER DESALINATION; FUEL-CELLS; DISTILLATION; REDUCTION; SURFACE; MACROMOLECULES
Abstract:
We propose a new approach to desalination of water whereby a pressure difference across a vapor-trapping nanopore induces selective transport of water by isothermal evaporation and condensation across the pore. Transport of water through a nanopore with saline water on one side and pure water on the other side under a pressure difference was theoretically analyzed under the rarefied gas assumption using a probabilistic framework that accounts for diffuse scattering from the pore walls as well as reflection from the menisci. The analysis revealed that in addition to salinity, temperature, and pressure difference, the nanopore aspect ratio and the probability of condensation of a water molecule incident on a meniscus from the vapor phase, known as the condensation coefficient, are key determinants of flux. The effect of condensation coefficient on mass flux becomes critical when the aspect ratio is small. However, the mass flux becomes independent of the condensation coefficien
t as the pore aspect ratio increases, converging to the Knudsen flux for long nanopores. For design of a nanopore membrane that can trap vapor, a minimum aspect ratio is derived for which coalescence of the two interfaces on either side of the nanopore remains energetically unfavorable. Based on this design criterion, the analysis suggests that mass flux in the range of 20-70 g/m(2) s may be feasible if the system is operated at temperatures in the range of 30-50 degrees C. The proposed approach further decouples transport properties from material properties of the membrane, which opens the possibility of engineering membranes with appropriate materials that may lead to reverse osmosis membranes with improved flux, better selectivity, and high chlorine resistance. (C) 2010 American Institute of Physics. [doi:10.1063/1.3419751]
Reprint Address:
Karnik, R, MIT, Dept Mech Engn, Cambridge, MA 02139 USA.
Research Institution addresses:
[Lee, Jongho; Karnik, Rohit] MIT, Dept Mech Engn, Cambridge, MA 02139 USA
E-mail Address:
karnik@mit.edu
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64
Times Cited:
0
Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA
Subject Category:
Physics, Applied
ISSN:
0021-8979
DOI:
10.1063/1.3419751
IDS Number:
650NV
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Title:
Stabilities and Electronic Properties of Ice Nanotube Encapsulated in Single-wall Carbon Nanotube
Authors:
Yang, BH; Zhang, AH; Li, L
Author Full Names:
Yang Baohua; Zhang Aihua; Li Lin
Source:
CHINESE JOURNAL OF CHEMISTRY 28 (7): 1076-1080 JUL 2010
Language:
English
Document Type:
Article
Author Keywords:
carbon nanotube; ice nanotube; self-consistent-field crystal orbital method; stability; electronic structure
KeyWords Plus:
WATER
Abstract:
The one-dimensional n-gon ice nanotube and its hybrid structure n-gon@(m,n) are investigated using ab initio self-consistent-field crystal orbital method based on density functional theory. The study focused on the stabilities and electronic properties of ice tube and n-gon@(m,n) complex. The results show that the pentagon and hexagon ice tubes are most stable and all the tubes are semiconductor with the band gap of -6 eV for the isolated ice nanotube. For the complex n-gon@(m,n), the interwall spacing between the carbon nanotube and ice tube plays an important role in the stabilities of resultant structures. The most stable complex has optimum interwall spacing which is close to the van der Waals distance. The frontier energy bands of n-gon@(m,n) complex are mainly derived from carbon nanotube and encapsulation of ice tube can not modulate the electronic properties of CNT.
Reprint Address:
Yang, BH, Capital Med Univ, Yanjing Med Coll, Beijing 101300, Peoples R China.
Research Institution addresses:
[Yang Baohua; Zhang Aihua; Li Lin] Capital Med Univ, Yanjing Med Coll, Beijing 101300, Peoples R China
E-mail Address:
y_b_h_@sohu.com
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Cited Reference Count:
18
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Multidisciplinary
ISSN:
1001-604X
DOI:
10.1002/cjoc.201090188
IDS Number:
653IV
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