Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
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Title:
Microfluidic Transport and Micro-scale Flow Physics: An Overview
Authors:
Chakraborty, D; Chakraborty, S
Author Full Names:
Chakraborty, Debapriya; Chakraborty, Suman
Source:
MICROFLUIDICS AND MICROFABRICATION : 1-85 2010
Language:
English
Document Type:
Proceedings Paper
Author Keywords:
Interfacial slip; slip length; Kundsen number; Reynolds number; capillary number; Bond number; continuum hypothesis; hydrophobic; interaction; nanobubble; friction factor; continuity equation; momentum; equation; Stokes hypothesis Navier Stokes equation; laminar flow; fully; developed flow; surface tension driven flow; contact angle; Young Laplace; equation; capillary filling; Marangoni effect; electrocapillary; continuous; electrowetting electrowetting on dielectric (EWOD); Young Lippman equation; optofluidics; rotational microfluidics (lab on a CD); electrokinetics; electrical; double layer (EDL); electroosmosis; streaming current; streaming potential; Poisson equation Poisson Boltzmann equation; steric effect; AC electroosmosis; electrophoresis; dielectrophoresis; electrothermal effect; electro-magnetohydrodynamics (EMHD); acoustic streaming; droplet based microfluidics
KeyWords Plus:
ELECTRIC DOUBLE-LAYER; HEAT-TRANSFER; LIQUID FLOW; ELECTROLYTE-SOLUTION; DRIVEN FLOW; FLUID-FLOW; MICROCHANNELS; WATER; DROPLET; WALL
Abstract:
In this article, we delineate some of the distinctive and demarcating fundamental aspects of microscale fluid flows as compared to their macroscale counterparts, and illustrate the utilization of these principles towards exploiting new functionalities in devices and systems of emerging importance. In particular, we emphasize on some of the important flow actuation mechanisms (pressure-driven, surface tension-driven, centrifugal, electrokinetic, magnetohydrodynamic, optical, and acoustic) in microfluidics and their implications, and outline the fundamental physical and mathematical principles that govern their implementations in practice.
Reprint Address:
Chakraborty, S, Indian Inst Technol, Dept Mech Engn, Kharagpur 721302, W Bengal, India.
Research Institution addresses:
[Chakraborty, Debapriya; Chakraborty, Suman] Indian Inst Technol, Dept Mech Engn, Kharagpur 721302, W Bengal, India
E-mail Address:
debapriya.chakraborty@gmail.com; suman@mech.iitkgp.ernet.in
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Cited Reference Count:
85
Times Cited:
0
Publisher:
SPRINGER; 233 SPRING STREET, NEW YORK, NY 10013, UNITED STATES
DOI:
10.1007/978-1-4419-1543-6_1
IDS Number:
BRA46
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Title:
Synthetic Chloride-Selective Carbon Nanotubes Examined by Using Molecular and Stochastic Dynamics
Authors:
Hilder, TA; Gordon, D; Chung, SH
Author Full Names:
Hilder, Tamsyn A.; Gordon, Dan; Chung, Shin-Ho
Source:
BIOPHYSICAL JOURNAL 99 (6): 1734-1742 SEP 22 2010
Language:
English
Document Type:
Article
KeyWords Plus:
BORON-NITRIDE NANOTUBES; BROWNIAN DYNAMICS; WATER TRANSPORT; FORCE-FIELDS; CHANNELS; SIMULATIONS; PERMEATION; CHEMISTRY; MEMBRANE; SEPARATION
Abstract:
Synthetic channels, such as nanotubes, offer the possibility of ion-selective nanoscale pores which can broadly mimic the functions of various biological ion channels, and may one day be used as antimicrobial agents, or for treatment of cystic fibrosis. We have designed a carbon nanotube that is selectively permeable to anions. The virtual nanotubes are constructed from a hexagonal array of carbon atoms (graphene) rolled up to form a tubular structure, with an effective radius of 4.53 angstrom and length of 34 angstrom. The pore ends are terminated with polar carbonyl groups. The nanotube thus formed is embedded in a lipid bilayer and a reservoir containing ionic solutions is added at each end of the pore. The conductance properties of these synthetic channels are then examined with molecular and stochastic dynamics simulations. Profiles of the potential of mean force at 0 mM reveal that a cation moving across the pore encounters an insurmountable free energy barrier of simil
ar to 25 kT in height. In contrast, for anions, there are two energy wells of similar to 12 kT near each end of the tube, separated by a central free energy barrier of 4 kT. The conductance of the pore, with symmetrical 500 mM solutions in the reservoirs, is 72 pS at 100 mV. The current saturates with an increasing ionic concentration, obeying a Michaelis-Menten relationship. The pore is normally occupied by two ions, and the rate-limiting step in conduction is the time taken for the resident ion near the exit gate to move out of the energy well.
Reprint Address:
Hilder, TA, Australian Natl Univ, Res Sch Biol, Canberra, ACT, Australia.
Research Institution addresses:
[Hilder, Tamsyn A.; Gordon, Dan; Chung, Shin-Ho] Australian Natl Univ, Res Sch Biol, Canberra, ACT, Australia
E-mail Address:
tamsyn.hilder@anu.edu.au
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Times Cited:
0
Publisher:
CELL PRESS; 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA
Subject Category:
Biophysics
ISSN:
0006-3495
DOI:
10.1016/j.bpj.2010.06.034
IDS Number:
654UY
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Title:
Water Chains in Hydrophobic Crystal Channels: Nanoporous Materials as Supramolecular Analogues of Carbon Nanotubes
Authors:
Natarajan, R; Charmant, JPH; Orpen, AG; Davis, AP
Author Full Names:
Natarajan, Ramalingam; Charmant, Jonathan P. H.; Orpen, A. Guy; Davis, Anthony P.
Source:
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 49 (30): 5125-5129 2010
Language:
English
Document Type:
Article
Author Keywords:
crystal engineering; hydrogen bonding; hydrophobic effect; supramolecular chemistry; water chains
KeyWords Plus:
TRANSPORT; MEMBRANES
Reprint Address:
Davis, AP, Univ Bristol, Sch Chem, Cantocks Close, Bristol BS8 1TS, Avon, England.
Research Institution addresses:
[Natarajan, Ramalingam; Charmant, Jonathan P. H.; Orpen, A. Guy; Davis, Anthony P.] Univ Bristol, Sch Chem, Bristol BS8 1TS, Avon, England
E-mail Address:
anthony.davis@bristol.ac.uk
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Cited Reference Count:
19
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Multidisciplinary
ISSN:
1433-7851
DOI:
10.1002/anie.201002418
IDS Number:
632NT
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